Based on what we know about diet soda's main components, here's how they stack up.Least Harmful? 	The newly reformulated Diet Pepsi no longer has aspartame—so that may push it to the top of the list. But it still contains acesulfame potassium (ace-K), which is poorly tested, although two studies suggest it may pose a cancer risk, as well as sucralose (Splenda), which the CSPI is now approaching with caution since the authors of a forthcoming study link it to leukemia. "The thing is, aspartame has undergone better cancer testing than these other artificial sweeteners," Lefferts explains, "so while it appears to be the worst from a risk perspective, it's possible that these others are just as bad and we just don't know it."

MORE: 8 Things That Happen When You Finally Stop Drinking Diet Soda Diet Pepsi also contains caramel color, which is not like caramel you might make at home by melting sugar in a saucepan. “The caramel color used in soda is made with ammonia and sulfites under high pressure and temperatures,” Lefferts explains. In the process, contaminants like a cancer-causing agent called 4-methylimidazole, or 4-MI, can form. The levels of 4-MI are much higher in Diet Pepsi than in Diet Coke, according to testing by Consumer Reports, although its most recent testing shows improvements. In 2011, the International Agency for Research on Cancer, an arm of the World Health Organization, concluded that 4-MI is “possibly carcinogenic to humans,” and California now lists it as a carcinogen. Consumer Reports’ testing has found that some sodas sold in California have much lower levels of 4-MI than the same brands sold in other states. Diet Coke with Splenda also carries no risks from aspartame, but the sweetness comes from sucralose, which is now on the caution list, per the CSPI, as well as ace-K, which is on CSPI’s avoid list. (Check out 57 sneaky names for sugar.)Somewhere in the Middle Aspartame is the go-to sweetener in most diet sodas, so regular drinkers might think twice about what they’re guzzling. Their aspartame content, in order from least to most per 8-ounce bottle: Sprite Zero (50 mg), Coke Zero (58 mg), Pepsi Max (77 mg), Diet Pepsi and Caffeine-Free Diet Pepsi (111 mg and 118 mg, respectively), Diet Dr. Pepper (123 mg), Diet Coke and Caffeine-Free Coke (125 mg). MORE: 4 Ways To Beat Your Diet Soda Addiction In One Week Keep in mind that all of them—except Sprite Zero—also contain caramel color and thus the potential for 4-MI. And unless they’re labeled as “caffeine-free,” the caffeine in these sodas can be a problem for children, pregnant women, and people sensitive to caffeine.The Worst Diet Mountain Dew may well be the riskiest diet soda because it has the greatest number of questionable additives. Not only does it contain aspartame, ace-K, and sucralose, but it also has more caffeine than most diet sodas, and it gets its color from yellow #5, which has been shown to cause hyperactivity in some children. As a kicker, Diet Mountain Dew also contains the emulsifier brominated vegetable oil (BVO), which has been shown to leave residues in body fat and the fat in the brain, liver, and other organs. The FDA in 1970 declared BVO not “generally recognized as safe,” but permitted its use on an interim basis pending additional study, and it hasn’t budged from that status since. PepsiCo and Coca-Cola have pledged to remove BVO from any of their drinks that contain it, but they didn’t say when that might happen.    MORE: 8 Things That Happen When You Quit Caffeine At the end of the day, Diet Pepsi’s reformulation without aspartame may just be one last-gasp effort by the diet soda industry to revive its flagging sales. More and more people are simply making healthier choices, including drinking low- and no-calorie beverages made without the worst of the sweeteners (like these delicious Sassy water recipes). A handful of examples: Steaz (sweetened with stevia and erythritol, a sugar alcohol that CSPI considers safe), DrinkMaple Pure Maple Water (with no added sugars, and half the natural sugar in coconut water), Reed’s Ginger Brews (the “light” version is sweetened with stevia leaf extract and honey), Hot Lips Pear Soda (with no added sugar), and Zevia Cola (made with erythritol, stevia extract, and monk fruit extract).